There is no official zip file for the PPSSPP emulator because the game was never released for the PlayStation Portable (PSP). God of War: Ascension was developed exclusively for the PlayStation 3 (PS3) and uses a significantly more powerful engine than the PSP could handle. Game Platform Information
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Yes, the PPSSPP emulator itself is legal and open-source. It is software designed to play games. The legality comes into question based on how you obtain the game files. There is no official zip file for the